Synthesis 2013; 45(4): 479-490
DOI: 10.1055/s-0032-1318100
paper
© Georg Thieme Verlag Stuttgart · New York

Thienopyrimidinedione Formation Versus Ester Hydrolysis from Ureido Carboxylic Acid Methyl Ester

Marie Reille-Seroussi
a   Université Paris Descartes, Sorbonne Paris Cité, CNRS UMR 8638, UFR Faculté des Sciences Pharmaceutiques et Biologiques, 4 avenue de l’Observatoire, 75270 Paris cedex 06, France   Fax: +33(1)43291403   Email: florent.huguenot@parisdescartes.fr
,
Raphaël Labruère
a   Université Paris Descartes, Sorbonne Paris Cité, CNRS UMR 8638, UFR Faculté des Sciences Pharmaceutiques et Biologiques, 4 avenue de l’Observatoire, 75270 Paris cedex 06, France   Fax: +33(1)43291403   Email: florent.huguenot@parisdescartes.fr
,
Nicolas Inguimbert
b   Université de Perpignan Via Domitia, Laboratoire de Chimie des Biomolécules, 52 avenue Paul Alduy, 66860 Perpignan, France
,
Sylvain Broussy
a   Université Paris Descartes, Sorbonne Paris Cité, CNRS UMR 8638, UFR Faculté des Sciences Pharmaceutiques et Biologiques, 4 avenue de l’Observatoire, 75270 Paris cedex 06, France   Fax: +33(1)43291403   Email: florent.huguenot@parisdescartes.fr
,
Nathalie Gagey-Eilstein
a   Université Paris Descartes, Sorbonne Paris Cité, CNRS UMR 8638, UFR Faculté des Sciences Pharmaceutiques et Biologiques, 4 avenue de l’Observatoire, 75270 Paris cedex 06, France   Fax: +33(1)43291403   Email: florent.huguenot@parisdescartes.fr
,
Wang-Qing Liu
a   Université Paris Descartes, Sorbonne Paris Cité, CNRS UMR 8638, UFR Faculté des Sciences Pharmaceutiques et Biologiques, 4 avenue de l’Observatoire, 75270 Paris cedex 06, France   Fax: +33(1)43291403   Email: florent.huguenot@parisdescartes.fr
,
Michel Vidal*
a   Université Paris Descartes, Sorbonne Paris Cité, CNRS UMR 8638, UFR Faculté des Sciences Pharmaceutiques et Biologiques, 4 avenue de l’Observatoire, 75270 Paris cedex 06, France   Fax: +33(1)43291403   Email: florent.huguenot@parisdescartes.fr
c   UF de Pharmacocinétique et Pharmacochimie, AP-HP, Hôpital Cochin, 75014 Paris, France   Email: michel.vidal@parisdescartes.fr
,
Florent Huguenot*
a   Université Paris Descartes, Sorbonne Paris Cité, CNRS UMR 8638, UFR Faculté des Sciences Pharmaceutiques et Biologiques, 4 avenue de l’Observatoire, 75270 Paris cedex 06, France   Fax: +33(1)43291403   Email: florent.huguenot@parisdescartes.fr
d   Université Paris Descartes, Sorbonne Paris Cité, UFR Biomédicale des Saints-Pères, 45 rue des Saints-Pères, 75270 Paris cedex 06, France
› Author Affiliations
Further Information

Publication History

Received: 10 October 2012

Accepted after revision: 20 December 2012

Publication Date:
17 January 2013 (online)


Abstract

The basic hydrolysis of ureidothienyl carboxylic esters was found to depend on the substitution pattern of the ureido moiety. While various hindered substituents led to carboxylic acid formation, unhindered substituents preferentially resulted in a cyclization step, yielding thienopyrimidinedione derivatives.

 
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